Effect of diisocyanate structure on thermal properties and microstructure of polyurethanes based on polyols derived from renewable resources

  • M. Angeles Corcuera
  • , Lorena Rueda
  • , Borja Fernández D'Arlas
  • , Ainara Saralegui
  • , Cristina Marieta
  • , Aitor Arbelaiz
  • , Iñaki Mondragon
  • , Arantxa Eceiza

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

1 Citation (Scopus)

Abstract

Polyols derived from renewables resources are good candidates to obtaining segmented polyurethane elastomers. Diisocyanates with different chemical structure, aliphatic and aromatic, have been used to synthesize by a two step polymerization procedure polyurethane elastomers with different hard segment content. Microphase separation and thermal stability have been studied using attenuated total reflection Fourier transform infrared spectroscopy (ATR-FTIR), differential scanning calorimetry (DSC) and thermogravimetric analysis (TGA). The analysis of the H-bonded and non H-bonded urethane carbonyl stretching vibration in the amide I region, the glass transition temperature of the soft and hard segments and the melting temperature and enthalpies of hard segment reveal that aliphatic diisocyanate based polyurethanes present higher phase separation degree and harder segment crystallinity and also superior thermal stability than aromatic diisocyanate-based polyurethanes.

Original languageEnglish
Title of host publicationVth International Conference on Times of Polymers (TOP) and Composites
Pages290-293
Number of pages4
DOIs
Publication statusPublished - 2010
Externally publishedYes
Event5th International Conference on Times of Polymers (TOP) and Composites - Ischia, Italy
Duration: 20 Jun 201023 Jun 2010

Publication series

NameAIP Conference Proceedings
Volume1255
ISSN (Print)0094-243X
ISSN (Electronic)1551-7616

Conference

Conference5th International Conference on Times of Polymers (TOP) and Composites
Country/TerritoryItaly
CityIschia
Period20/06/1023/06/10

Keywords

  • Castor oil
  • Microphase structure
  • Polyurethane
  • Thermal properties

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