Pore flow-through catalytic membrane reactor for steam methane reforming: characterization and performance

M. Angulo*, I. Agirre, A. Arratibel, M. A. Llosa Tanco, D. A. Pacheco Tanaka, V. L. Barrio

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

1 Citation (Scopus)

Abstract

A series of pore flow-through catalytic nonselective membrane reactors (PTCMRs) were studied for steam methane reforming (SMR) in the 500 to 900 °C temperature range under 10 barg pressure and a steam-to-carbon ratio of 5. The reactants flow through the pores of the membrane where they react on contact with the Pd nanoparticles. Various reactor configurations were prepared and tested with porous α-Al2O3-based ceramic tubes with one or more γ-Al2O3/YSZ layers on the external surface. The palladium content and dispersion affect the catalytic activity of the reactors and the results show that the efficiency of the reactions depends on the number of γ-Al2O3/YSZ layers.

Original languageEnglish
Pages (from-to)2240-2253
Number of pages14
JournalReaction Chemistry and Engineering
Volume7
Issue number10
DOIs
Publication statusPublished - 12 Jul 2022

Funding

University of the Basque Country (UPV/EHU) and the Basque Government (IT993-16 & MALTA KK-2017/00051) supported this work. The authors also acknowledge the contribution of Prof. Cambra (retired).

FundersFunder number
Eusko JaurlaritzaMALTA KK-2017/00051, IT993-16
Euskal Herriko Unibertsitatea

    Keywords

    • Alumina
    • Aluminum oxide
    • Bioreactors
    • Catalyst activity
    • Catalytic reforming
    • Methane
    • Palladium

    Project and Funding Information

    • Funding Info
    • University of the Basque Country (UPV/EHU) and the Basque Government (IT993-16 & MALTA KK-2017/00051) supported this work. The authors also acknowledge the contribution of Prof. Cambra (retired).

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